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Meeting MS&T23: Materials Science & Technology
Symposium Energy Materials for Sustainable Development
Presentation Title Deep Learning Tomography Reconstruction of Lithium Ion Battery Defects: Providing High Resolution at Large Length Scales
Author(s) Nathan S. Johnson, Yulia Trenikhina, Hrishi Bale, William Harris, Steve Kelly
On-Site Speaker (Planned) Nathan S. Johnson
Abstract Scope Successfully manufacturing lithium-ion batteries necessitates tailoring material properties across various length scales. Defects in lithium-ion particle fabrication occur at nanometer scales, porosity between battery layers can emerge at micron scales, and cracks in the device can span up to millimeters. Effectively imaging all defects in a device demands the collection of multiple datasets at different length scales and often the use of multiple imaging techniques. In this study, we demonstrate the application of deep learning to generate X-ray tomography datasets that cover large volumes (from millimeters to microns) while providing high resolution (from microns to nanometers). This technique is employed to detect porosity and discontinuities in the Cu charge-collecting layer of a lithium-ion battery device. Although these defects are too small to observe at the millimeter scale, they are easily discerned at the micron scale. We showcase that deep learning reconstruction can enhance the resolution of datasets, enabling the detection of these defects at the millimeter scale. The presence, size, and morphology of the defects are verified using separate independent X-ray tomography scans at high resolution, as well as through scanning electron microscopy. Furthermore, we discuss the limitations of this technique and provide a preview of its application on other sustainable energy materials, such as solid oxide fuel cells and additional solid-state battery devices.

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

A Study of the Role of Molten Salt Treatment in the Observed Improved Water Splitting Ability of SrTiO3
Accelerated Investigation of Electrocatalysts with Integrated Computational Approaches
Application of Coal-derived Graphites as Lithium-ion Battery Anodes
Cation-Driven Assembly of Dissimilar Nanoflakes to Form Two-dimensional Heterostructure Electrodes for Energy Storage
Ceramics Nanocomposite Materials for Novel Energy Harvesting and Heat Management
Charge Storage Mechanisms in Layered Oxide Supercapacitors
Deep Learning Tomography Reconstruction of Lithium Ion Battery Defects: Providing High Resolution at Large Length Scales
Developing Fast Chargeable Safe and Inexpensive Li-ion Batteries
D.T. Rankin Award Ceremony and Awardee’s Talk
Electrically Conductive Electrets as a New Untapped Source of Electrical Energy
Facile Routes to Synthesis Electrochemical Energy Storage Materials and Their Patterned Deposition to Construct Planar Micro-supercapacitors
Ferroelectric Nanocomposites for Enhanced Solar Energy Conversion
High Thermoelectric ZT in Half-Heusler Alloys: A Preview
Metal Composite Nano-Catalysts for Enhanced Solid Oxide Fuel Cell Operation and Stability within Hydrocarbon Containing Fuels
Modeling and Performance Evaluation of Barocaloric Refrigeration
O-10: Electron Transfer Mechanism of Near-infrared-response ZnO/CuInS2 S-scheme Photocatalyst for H2O2 Synthesis and Glycerol Oxidation
O-11: Smart Shoe Electricity Generation via Piezo-electric Transducers
O-7: Bandgap-engineered Ferroelectric Ceramics for Photoelectric and Photovoltaic Applications
O-8: Bimetallic Indium-Tin Metal-Organic Framework Catalyst for CO2 Conversion to Formic Acid
O-9: Computational Modeling of Correlated Ion Transport in Polymer-Ceramic Composite Electrolytes
Oxide-halide Perovskite Composites for Simultaneous Recycling of Piezoceramics and Solar Cells
Performance Improvement of MXene-based Perovskite Solar Cells
Processing and Characterization of Epitaxial Cathode-electrolyte Interfaces in All-solid-state Thin-film Lithium-ion Batteries
Processing and Performance of High Entropy Oxide as Anodes for Lithium-ion Batteries
Superconductors and Cryogenic Conductors for Electric Aircraft Propulsion Systems
Synergistic Photothermal-thermoelectric-photovoltaic Energy Generation via Transparent Nanohybrids of Porphyrin and Iron Oxide
Tailoring the Sulfur Electrode for Enhanced Kinetics and Longevity of Li-S Batteries
Texturing Ca3Co4-xO9-δ Ceramics via Electrospun Nanoribbons: A Route to High-performance Thermoelectrics
The Effect of A-site Doping Elements and Concentrations on the Diffusivity and Ionic Conductivity of La2NiO4+δ Studied by Ab Initio Calculations
Towards Designing Mn- and Fe-rich Cathode Materials in Sodium-ion Batteries
Twin Perovskie Nanocomposite Cathodes for High-Performance Protonic Ceramic Fuel Cells

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