Uranium electrodeposits, extracted in LiCl-KCl eutectic, were studied under varied overpotentials (25 mV, 50 mV, 100 mV, 200 mV) and molten salt weight concentration ratios of uranium to cerium (1:0, 1:1, 2:1) to investigate their effects on the morphology and chemical composition (purity) of the reduced uranium metal. Scanning electron microscopy with energy dispersive spectroscopy (SEM-EDS) capabilities was used to characterize the morphology and elemental surface composition of the collected uranium metal samples. Inductively coupled plasma mass spectrometry (ICP-MS) and x-ray diffraction (XRD) techniques were utilized for determining the overall composition of those samples. For the studied conditions, the final chemical compositions of the uranium electrodeposits indicate no correlation with varying the concentration ratios or overpotential, whereas morphology is greatly influenced with applied overpotential. A relationship between electrolytic time, electroactive working electrode surface area, and applied overpotential and their combined effect on electrodeposit growth is proposed and will be discussed.