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Meeting 2027 TMS Annual Meeting & Exhibition
Symposium Hume-Rothery Symposium: Data-Driven Materials Discovery and Phase Stability
Presentation Title Computational Design of Battery Guided by Degradation Mechanism
Author(s) Hyungjun Kim
On-Site Speaker (Planned) Hyungjun Kim
Abstract Scope The transition toward sustainable energy and electrified transportation has made high-performance secondary batteries essential to modern technology. Yet the development of next-generation energy storage materials remains constrained by conventional trial-and-error experimentation, which cannot keep pace with the coupled multiphysics phenomena—such as chemical degradation, mechanical failure, and thermal instability—that govern battery performance. Here, we present a computation-driven design framework that couples multiscale simulation with artificial intelligence to accelerate the discovery and optimization of advanced battery materials. First, we employ multiscale modeling spanning atomistic to continuum scales to clarify degradation pathways, revealing how structural distortion and misalignment across particle length scales generate inhomogeneous stress and drive capacity loss. These insights inform rational strategies for improving both ionic transport and mechanical durability. Second, we combine high-throughput screening with explainable machine learning to navigate vast material spaces, identifying key physical descriptors that govern stability and guiding the design of next-generation electrode materials.
Proceedings Inclusion? Planned:
Keywords Computational Materials Science & Engineering, Energy Conversion and Storage, Modeling and Simulation

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

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Atomic-Scale Simulations of Metal/Molten-Salt Interfaces by Machine-Learning Interatomic Potentials
Beyond Order: A Disorder-Aware Workflow toward OQMD 2.0
Beyond Randomness: Designing Short-Range Order for Materials Performance
Bonding-Driven Discovery and Design of Thermoelectric Materials
Calibrated Machine-Learning Uncertainty for Data-Driven Alloy Design
Chemical Intuition as a Guide to Data-Driven Materials Discovery
Computational Design of Battery Guided by Degradation Mechanism
Computational discovery of materials for energy storage
Data- and Simulation-Driven Design of Structural and Functional Materials: Successes and Challenges
Data-Driven Discovery of Novel High-Performance Photovoltaics in an Experimentally Known Family of Quaternary Chalcogenides
Data-driven Prediction of Solid-State Synthesis
Elemental Features for Data-Driven Materials Properties Prediction
Elucidating the role of solute-solute interactions on diffusion in Ni-based substitutional solid solutions
Exploring the electronic structure of all known inorganics - from transport to superconductivity to topology.
First-principles modeling of disorder in cathodes and beyond
From Computational Design to Accelerated Discovery of High-Entropy Alloys
Functional Synthesizability: Tuning the Extreme-Properties of High-Entropy Ceramics
High-Throughput Anharmonic Phonons for Data-Driven Materials Discovery, Phase Stability, and Thermal Transport
How Computational Modeling Shapes Materials at Apple
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Integrating Automated Computation with Experiment for Accelerated Materials Discovery
Irreversible Thermodynamic Basis for the Phase-field Method of Ordered Stoichiometric Compounds
Lithium Extraction with Ion Exchange at Lilac Solutions
Mapping Lithium-Ion Transport in Sulfide Argyrodites: From Defect Chemistry to Composite Interfaces
Phase Diagrams On-Demand
Relationship Between Configurational and Vibrational Entropies of Mixing and Their Effects on Phase Diagrams
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Symmetry Broken DFT Corrects the Stability and Mott Band Gap Errors Without Adding Strong Correlations
The Generalized Aliasing Decomposition, A New Paradigm for Modeling
The Possibility of New Complex Magnet Material
The Spatial Arrangement of Nanoparticles on Substrates and the Role of Phase Transformations
Theoretical Insights Into Hydrogenation and Proton Transport in ABO3 Perovskite
Thermodynamic and Kinetic Stability of M–N–C Active Sites for O₂ Reduction
Towards Ai-enabled High Throughput Characterization and Materials Discovery
Zentropy: A Thermodynamic Framework Bridging Phase Stability, Data-Driven Modeling, and Artificial Intelligence

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