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Meeting MS&T26: Materials Science & Technology
Symposium Advances in Emerging Electronic Nanomaterials: Towards Next-Generation Microelectronics
Presentation Title Atomic-Resolution Imaging of Ferroelectric Domains in Emerging Fluorite-Type Ferroelectrics
Author(s) Ece Gunay, Sebastian Calderon, Rintaro Maki, Yuichi Shimakawa, Daisuke Kan, Elizabeth Dickey
On-Site Speaker (Planned) Ece Gunay
Abstract Scope Logic-in-memory architectures reduce the energy cost of data-intensive computing by combining computation and storage, but they require scalable ferroelectric materials compatible with CMOS technology. Y-doped hafnium oxide is a promising candidate because yttrium stabilizes the metastable ferroelectric orthorhombic phase. To probe nanoscale structures and domain configurations that govern device performance, freestanding Hf0.93Y0.07O2 membranes with predominantly in-plane polarization were prepared for atomic-resolution characterization. Using aberration-corrected scanning transmission electron microscopy (STEM), we identified nanoscale tetragonal-like inclusions preferentially located near grain boundaries and 90° domain walls. These heterogeneities preserve the overall lattice while exhibiting local in-plane distortions that influence the functional properties and reliability of hafnia-based emerging ferroelectrics. (This material was based upon work supported by the Center for 3D Ferroelectric Microelectronics Manufacturing (3DFeM2), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers program under Award Number DE-SC0021118.)

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

4D-STEM and Machine Learning for Nanoscale Structure-Property Mapping in Emerging Electronic Materials
A General Process to Produce Large-Size Single Crystal Room-Temperature Diluted Magnetic Semiconductors
Atomic-Resolution Imaging of Ferroelectric Domains in Emerging Fluorite-Type Ferroelectrics
Bio-Inspired Event-based Infrared Vision Enabled by Colloidal Quantum Dots
Effects of Ta Crystalline Phase on Ultrathin TaOx Neuromorphic Devices
Electronics Enabled by Mechanical Metamaterials
Engineered Transparency and Conductivity of IZO/Ag/IZO Multilayers by Intense Pulsed Light for Perovskite Solar Cells
Fabrication and Characterization of SnO2/CdS Quantum Dots Heterojunction for UV-Vis Sensitive Low-Voltage Phototransistors
Heterogeneous Integration Using Freestanding Gallium Nitride Membranes
Inverse-Designed 3D Holographic Lithography for Next-Generation Microelectronic Architectures
Ion Beam Treatment to Control Properties of Two-Dimensional Semiconductors
Large-Scale, Crack-Free Oxide Membranes for Tunable Twistronics
Laser-Engineered Graphene Composites for Emerging Electronic Nanomaterials
Metal Nanowire-Based Electrodes and Their Applications in Optoelectronics and Bioelectronics
Mxene-enabled Micro-Battery Architectures for Advanced Semiconductor Devices
Scaling and Integration of Hafnia-Based Ferroelectrics for High-Density and Neuromorphic Applications
Spatiotemporal Laser Control of Iron-Oxide-Nanoparticle-Integrated Graphene Microelectrodes for Bioelectronic Sensing
Sub-5nm Thick Plasma-Enhanced Atomic Layer Deposited Indium Oxynitride Channel Transistor for 3D Monolithic Device Applications
Thermodynamic Modeling and CVD Synthesis of Mo, Nb, and V MXene Precursors
Topological Semimetal and Single-Crystalline Cu for Overcoming Resistivity Scaling in Nanoscale Interconnects
Toward Controlled Synthesis of 2D Materials: Data-Driven Modeling of ALD Growth Mechanisms
Wafer-Scale 2D Semiconductors Integrated on Arbitrary Substrates for Emerging Optoelectronic Artificial Synapses with Flexoelectricity
Field Gradient Engineering of van der Waals Semiconductors

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