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Meeting MS&T26: Materials Science & Technology
Symposium Molecular Approaches to Ceramics; Synthesis, Processing, Modeling, and Derived Ceramics
Presentation Title Phase Evolution Study of Polymer Derived SiC and TiC-SiC Composites Under Ultrafast Heating
Author(s) Kishore Behera, Kathy Lu, Kartik Nemani, Shilpa Cholayil
On-Site Speaker (Planned) Kishore Behera
Abstract Scope Polymer-derived ceramics (PDCs) have attracted great attention for high-temperature sensing and structural applications because of their thermal stability, oxidation resistance, and ability to form high entropy compositions from liquid polymer precursors. In this work, ultrafast high-temperature heating has been used to study the phase evolution of SMP-10-derived SiC and SMP-10 derived SiC/Ti3C2Tx MXene composites. The materials are processed at temperatures between 1100 and 2000 °C using Joule-heated carbon felt, where the target temperatures are reached within seconds. Ti3C2Tx flakes are preserved within the amorphous SiC matrix up to 1300 °C, where they act as heterogenous nucleation sites for β-SiC crystallization. At 1600 °C, MXene undergoes topotactic conversion into TiC platelets surrounded by SiC grains, and at 2000 °C, a β-SiC/TiC nano composite is formed. The ultrafast heating suppresses MXene decomposition up to temperature 1300 °C and forms novel TiC-SiC composites within seconds from polymer derived ceramic precursor.

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

A ReaxFF Force Field for Atomistic Simulation of Tantalum Carbide Formation via Reactive Sputtering and Polymer Pyrolysis
A Systematic Approach to Enhancing the Oxidation Resistance of C/C Composites Using Multi-Layer SiC–ZrB₂-Based Coatings
Additive Manufacturing of Variable-Composition and Difficult-to-Print Ceramics Based on Preceramic Polymers
Advances in Materials for Extreme Environment Applications
Advances in the Processing of Ceramic Matrix Composites (CMCs) by Polymer Infiltration and Pyrolysis (PIP)
Building a PDC Genome: AI-Assisted Extraction and Gap Analysis of Preceramic Polymer Descriptors
Characterization of Processing-Induced Stress and Crack Formation in Polymer-Derived Ceramics During Pyrolysis
Chemical and Structural Evolution of MXene-SiOC Under Ground- and Micro-Gravity and Controlled Atmospheres
Deep Learning-Based Framework for ReaxFF Development in Reactive Material Systems
Design and Manufacturing of New Functional Ceramic Composites
Development and Application of ReaxFF Reactive Force Fields to Ceramics Synthesis and High-Temperature Ceramics Response
Development of a ReaxFF Reactive Force Field for the Investigation of Thermochemical, Thermophysical and Oxidation Behavior of Titanium Diboride
Development of MS-154 as a Lower-Cost Preceramic Polymer Route for SiC-Containing Ceramics
Development of the ReaxFF Reactive Force Field for Zirconium Carbide Ceramic Formation During Sputtering
Engineering with Carbosilane
From Single-Source Precursors to Compositionally Complex (Hf-Ti-Nb-W-V)CN Carbonitrides
Improved Electrochemical Stability of Lithium–Sulfur Batteries Using SiBCN Sulfur Hosts
Kinetics of Pyrolysis Measured During In-Situ Creep Experiments
Lignin-Silicon Hybrid Ceramic Structures: Chemically Active versus Passive Colloids in Preceramic Sol-Gel Systems
Molecularly Engineered Refractory-Metal Preceramic Inks for Printable Ultrahigh-Temperature Ceramic Coatings
Nanoscale Structural Evolution in Polycarbosilane-Derived Ceramics
Phase Evolution Study of Polymer Derived SiC and TiC-SiC Composites Under Ultrafast Heating
Photo-Rheology of Ceramic-Filled Preceramic Polymers for Material Extrusion Additive Manufacturing
Polymer-Derived SiTiOC Ceramics for Enhanced Polysulfide Confinement in Lithium–Sulfur Cells
Processing and Pyrolysis Effects in Polymer Derived Ultra-High Temperature Ceramics
Tailoring Polymer Grafted Nanoparticle Properties Via Modification of Polymer Structure and Nanoparticle Composition
The Influence of Residual Copper Catalyst on the Polymer-to-Ceramic Conversion of a Click-Derived Polycarbosilane
Understanding Pyrolysis of Polymer-Derived Carbonitrides Through Ab Initio-Based Machine Learning Interatomic Potential
Use of Embedded Oxidation Marker Particles to Track Oxidant Ingress in Heterogeneous Microstructures Produced from Polymer Derived Ceramics
Visualizing Polymer to Ceramic Transformations in SiOC Polymer Derived Ceramics with In Situ Transmission Electron Microscopy

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