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Meeting MS&T26: Materials Science & Technology
Symposium Molecular Approaches to Ceramics; Synthesis, Processing, Modeling, and Derived Ceramics
Presentation Title Additive Manufacturing of Variable-Composition and Difficult-to-Print Ceramics Based on Preceramic Polymers
Author(s) Apoorv Kulkarni, Thomas Lacelle, Hamidreza Yazdani Sarvestani, Chakavak Nojavan, Yadienka Martinez-Rubi, Amelie Robitaille, Behnam Ashrafi, Michael Jakubinek
On-Site Speaker (Planned) Michael Jakubinek
Abstract Scope Preceramic polymers enable both the use of polymer processing and shaping methods, and molecular-level control over the composition of the resulting polymer-derived ceramics (PDCs). While slurry-based 3D printing methods – using high-resolution printing approaches based on photopolymerization with ceramic particle suspensions in a sacrificial resin binder – are highly effective for ceramics such as alumina, a PDC approach can be advantageous for compositional flexibility, lower processing temperature, and for dark ceramics, which are challenging to produce by such methods. Here we show high-resolution 3D printing of preceramic polymers using digital light processing to achieve ceramic structures with complex gyroid geometries. A range of compositions will be discussed, including silicon-based, non-oxide (low oxygen content) ceramics. The structures exhibit fine features, low porosity, high temperature stability and good performance under compression, demonstrating the potential of the approach to target a broad range of difficult-to-print ceramic compositions.

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

A ReaxFF Force Field for Atomistic Simulation of Tantalum Carbide Formation via Reactive Sputtering and Polymer Pyrolysis
A Systematic Approach to Enhancing the Oxidation Resistance of C/C Composites Using Multi-Layer SiC–ZrB₂-Based Coatings
Additive Manufacturing of Variable-Composition and Difficult-to-Print Ceramics Based on Preceramic Polymers
Advances in Materials for Extreme Environment Applications
Advances in the Processing of Ceramic Matrix Composites (CMCs) by Polymer Infiltration and Pyrolysis (PIP)
Building a PDC Genome: AI-Assisted Extraction and Gap Analysis of Preceramic Polymer Descriptors
Characterization of Processing-Induced Stress and Crack Formation in Polymer-Derived Ceramics During Pyrolysis
Chemical and Structural Evolution of MXene-SiOC Under Ground- and Micro-Gravity and Controlled Atmospheres
Deep Learning-Based Framework for ReaxFF Development in Reactive Material Systems
Design and Manufacturing of New Functional Ceramic Composites
Development and Application of ReaxFF Reactive Force Fields to Ceramics Synthesis and High-Temperature Ceramics Response
Development of a ReaxFF Reactive Force Field for the Investigation of Thermochemical, Thermophysical and Oxidation Behavior of Titanium Diboride
Development of MS-154 as a Lower-Cost Preceramic Polymer Route for SiC-Containing Ceramics
Development of the ReaxFF Reactive Force Field for Zirconium Carbide Ceramic Formation During Sputtering
Engineering with Carbosilane
From Single-Source Precursors to Compositionally Complex (Hf-Ti-Nb-W-V)CN Carbonitrides
Improved Electrochemical Stability of Lithium–Sulfur Batteries Using SiBCN Sulfur Hosts
Kinetics of Pyrolysis Measured During In-Situ Creep Experiments
Lignin-Silicon Hybrid Ceramic Structures: Chemically Active versus Passive Colloids in Preceramic Sol-Gel Systems
Molecularly Engineered Refractory-Metal Preceramic Inks for Printable Ultrahigh-Temperature Ceramic Coatings
Nanoscale Structural Evolution in Polycarbosilane-Derived Ceramics
Phase Evolution Study of Polymer Derived SiC and TiC-SiC Composites Under Ultrafast Heating
Photo-Rheology of Ceramic-Filled Preceramic Polymers for Material Extrusion Additive Manufacturing
Polymer-Derived SiTiOC Ceramics for Enhanced Polysulfide Confinement in Lithium–Sulfur Cells
Processing and Pyrolysis Effects in Polymer Derived Ultra-High Temperature Ceramics
Tailoring Polymer Grafted Nanoparticle Properties Via Modification of Polymer Structure and Nanoparticle Composition
The Influence of Residual Copper Catalyst on the Polymer-to-Ceramic Conversion of a Click-Derived Polycarbosilane
Understanding Pyrolysis of Polymer-Derived Carbonitrides Through Ab Initio-Based Machine Learning Interatomic Potential
Use of Embedded Oxidation Marker Particles to Track Oxidant Ingress in Heterogeneous Microstructures Produced from Polymer Derived Ceramics
Visualizing Polymer to Ceramic Transformations in SiOC Polymer Derived Ceramics with In Situ Transmission Electron Microscopy

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