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Meeting 2027 TMS Annual Meeting & Exhibition
Symposium Interstitial–Metal Interactions: The Outsized Role of Small Atoms
Presentation Title Oxygen-mediated phase decomposition in group IV–Nb refractory alloys
Author(s) Israel Reimer, Arturo Zuniga, Daniel Bolden, Ravit Silverstein
On-Site Speaker (Planned) Israel Reimer
Abstract Scope Refractory multi-principal-element alloys (RMPEAs) show promise for next-generation high-temperature applications, yet their high ductile-to-brittle transition temperatures limit deployment. Recent studies have shown that dilute oxygen additions raise a miscibility gap in Ti-Nb, motivating investigation of analogous thermodynamic behavior across the Group IV-Nb series. These binary systems (TiNb, ZrNb, HfNb) provide an ideal model platform for isolating the role of Group IV chemistry in governing oxygen solubility, phase stability, and decomposition kinetics, thereby establishing design principles directly applicable to complex RMPEAs. This study systematically characterizes oxygen-mediated phase decomposition across the Group IV-Nb series as a function of alloy composition, oxygen content, and annealing conditions (800-1400 °C). The underlying mechanisms are investigated by correlating chemical partitioning, phase transformations, and microstructural evolution using multidimensional diffraction analysis (4D-STEM), coupled with unsupervised machine learning approaches and complementary chemical analysis. The implications for oxygen-driven phase stability and microstructural evolution in refractory alloys are discussed.
Proceedings Inclusion? Planned:
Keywords High-Temperature Materials, Phase Transformations, Characterization

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Coupled Effects of Hydrogen, Grain Boundaries, and Free Surfaces on Dislocation Activity in Polycrystalline Nickel
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Effects of Heat Treatment and Hydrogen Exposure on Fracture Resistance and Fatigue Crack Growth in 15-5 PH Stainless Steel
Effects of Interstitial Oxygen on the Grain-scale Deformation Behavior of Vanadium
Effects of Oxygen Interstitials on Vacancy Mobility in Refractory Metals and Alloys
Fracture Mechanics Evaluation of High-Pressure Torsion-Processed DSN9 Steel for Hydrogen–Natural Gas Pipeline Applications
Hydrogen-Vacancy Co-Segregation and Fast Grain-Boundary Hydrogen Diffusion in Copper
Hydrogen charging at room temperature to reduce dislocations in steel with residual stresses
Impact of Surface Oxide on Hydride Formation in Niobium and Tantalum
Influence of Hydrogen on Disconnection Energetics and Grain Boundary Migration in Nickel
Interstitial Diffusion in Grain Boundaries
Interstitial effects on temperature-dependent critical stress and dislocation glide of screw and edge dislocations in tantalum
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Microstructure-Controlled Hydrogen Trapping and TiH₂-Assisted Comminution of Ti-6Al-4V Machining Chips
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Oxygen-mediated phase decomposition in group IV–Nb refractory alloys
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The effect of hydrogen concentration on the monotonic and cyclic deformation behavior of <001> oriented pure nickel single crystal
Thermodynamics and Kinetics of Interstitials in TiZrHfNbTa Refractory High-Entropy Alloys
Time-scale Competition of Hydrogen–Defect Interactions: A Phase–Field Crystal Study
Tracking interstitial hydrogen atoms in metals by using atom probe tomography
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