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Meeting 2025 TMS Annual Meeting & Exhibition
Symposium Neutron and X-ray Scattering in Materials Science and Engineering
Presentation Title Probing Ionic Diffusion with Single Crystal Diffuse and Quasielastic Neutron Scattering
Author(s) Stephan Rosenkranz, Jared Coles, Raymond Osborn, Matthew Krogstad, Daniel Pajerowski
On-Site Speaker (Planned) Stephan Rosenkranz
Abstract Scope Cooperative motion of correlated ions has long been known to affect the conductivity of solid-state ion conductors. But a detailed understanding of correlated diffusion, microscopic diffusion pathways, residence times, activation energies, and the interplay between mobile ions and local relaxations of the surrounding lattice, required for optimizing the ionic conductivity, remains lacking. Quasi-elastic neutron scattering (QENS) and single crystal diffuse scattering can provide detailed insight into these local correlations and their dynamics. Such measurements can now be performed on single crystals providing coverage over four-dimensional momentum and energy transfer space, allowing detailed, quantitative comparison to jump diffusion models, such as the Chudley-Elliot model. We will discuss our analysis of 4D-QENS and diffuse scattering data from SrCl2, which reveals de Gennes narrowing of linewidths in regions of strong coherent scattering and provides evidence of the metastability of interstitial sites along the pathways. Work supported by the U.S. DOE, BES, DMSE
Proceedings Inclusion? Planned:
Keywords Other,

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

Anomalous Neutron Nuclear-Magnetic Interference Spectroscopy
Application of energy-dispersive X-ray diffraction for engineering alloys
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Characterization of Radiation Effects in Ceramics with Neutron Total Scattering
Effects of Cooling Rates on Residual Stress Evolution Quantified via Neutron Diffraction in Lubricant-free, Solid-state Repaired AA7075
Elucidating the phase evolution of a spinodal Au-Pt-Pd alloy using in situ synchrotron X-ray diffraction
Enhanced magnetic-disorder driven magnon softening of TbSb via Y-doping
Feasibility of a Focusing Small-Angle Neutron Scattering (SANS) Instrument at the MIT Nuclear Reactor Laboratory
From Angstroms to Micrometers: Across-length-scale Structural Characterization of Hard Materials via X-ray Scattering
HIPPO meets ERNI & BERT – Upgrading a neutron diffractometer with an energy-resolved neutron imaging detector
Impact of electric fields on local structure, phonons, and thermal transport in a relaxor ferroelectric
In-situ and multimodal capabilities of Laue diffraction instrument at 34-ID-E of the Advanced Photon Source
In-situ characterization of phase transformation dynamics in fusion-based metal additive manufacturing processes by high-speed X-ray diffraction
In situ X-ray diffraction reveals the early stages of solid phase alloying in the 7XXX Al alloy system
Influence of Selective Laser Preheating on Residual Stress in Ti-6Al-4V Laser Powder Bed Fusion (LPBF)
Investigating Thermal Transport in Nuclear Materials Using Neutron Scattering
Load Partitioning in Eutectic and Near-eutectic Ni-Ce Alloys
Machine Learning Models For X-ray Diffraction Temperature Inference
Mapping of the local residual stress in 316L stainless steel processed by laser powder bed fusion
Measurement of Residual Stress in Additively Manufactured Ti-6Al-4V & Ti-6Al-2Sn-4Zr-6Mo Walls using Neutron Diffraction
Operando inelastic neutron scattering measurements of glass dynamics
Operando X-ray and neutron diffraction and imaging during laser powder bed fusion
Overview of science capabilities of VENUS neutron imaging beamline at the Spallation Neutron Source at Oak Ridge National Laboratory
Phonon Dynamics and Thermal Transport in Tl3VSe4
Planar thermal transport mapping of the GaN film with Spatial-Temporal-Resolved X-ray diffraction
Probing Ionic Diffusion with Single Crystal Diffuse and Quasielastic Neutron Scattering
Rationalization of non-uniform radial hardness distribution in friction self-piercing riveted Al-7075 using x-ray scattering and advanced microscopy techniques
Redistribution of Residual Stress in Steels during Hybrid Manufacturing
Residual Strain Monitoring by Neutron Diffraction in Metal Additive Manufacturing
Scattering study of spin-lattice interactions in chromia
The development of a stress-strain diffractometer at the MIT Reactor using a polychromatic beam
The influence of grain size on the deformation-induced martensitic transformation in austenitic steels: from grain-average to single-grain behavior studied by in-situ high-energy synchrotron X-ray diffraction.
The Invar Effect Explained by Nuclear Resonant X-ray Scattering from Phonons and Spins
The Role Of Annealing And Grain Boundary Controls On The Mechanical Properties Of Limestones, Marbles And Novaculite
The Role of Vibrational Entropy Across Magnetostructural Transition in Heusler Alloys
The use of neutron diffraction for the understanding of additive manufacturing process of magnesium alloys
Time resolved synchrotron X-ray diffraction study of the structural and mechanical evolutions within a zirconium alloy oxidized at high temperature
Unveiling multiscale structure and dynamics with neutron imaging
Vibrational thermodynamics of the giant elastocaloric effect in NiCoMnTi alloys

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