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Meeting MS&T26: Materials Science & Technology
Symposium Advances in Refractory High Entropy Alloys and Ceramics
Presentation Title Dominant Role of Second Nearest-Neighbor Bonding in Strength-Ductility Tradeoff of bcc Refractory High Entropy Alloys
Author(s) Dharmendra Pant, Suyash Varshney, Dilpuneet S. Aidhy
On-Site Speaker (Planned) Dilpuneet S. Aidhy
Abstract Scope Balancing strength and ductility in BCC refractory high entropy alloys (RHEAs) remains a fundamental challenge due to the intrinsic trade-off between bond strength and dislocation mobility. Using (DFT) calculations, we show that there is a noticeable decrease in the density of states at the Fermi level, N(Ef), within a short window of valence electron concentration (VEC) around 5.1 marking a crossover from metallic to covalent-type bonding in refractory bcc alloys. This change is driven by a disproportionate suppression of eg states, responsible for σ-type bonds along second nearest neighbor (2NN) directions, relative to t2g states. The resulting increase in 2NN stiffness outpaces the increase in the first nearest neighbor (1NN) stiffness and drives steep rise in Young’s and shear moduli, while simultaneously reducing local lattice distortion and ductility. Enrichment with higher-VEC Group VI elements amplifies these effects, whereas addition of lower-VEC Group IV and V elements reduces them.

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

A Multiscale Modeling Study of the Mechanical Response of W-Mo Alloys
A Nanoindentation Study of Incipient Plasticity in Refractory High-Entropy Alloys
Compositional Emptiness as a Guide to Alloy Discovery
Defect-Controlled Oxidation Resistance of (Ln, U)O2 solid solutions Probed by XAFS and XRD
Design and Validation of Tungsten-Based High Entropy Alloys
Design of Heterostructured Refractory Alloys for High Temperature Applications
Dislocation Properties in Refractory Compositionally Complex Alloys
Dominant Role of Second Nearest-Neighbor Bonding in Strength-Ductility Tradeoff of bcc Refractory High Entropy Alloys
Dynamic Behavior of NbTaTiHf High-Entropy Alloy
Multidimensional Diffraction Insights into Oxygen-Amplified Strengthening in BCC Refractory Alloys
Nb-Regulated Selective Oxidation in Al–V–Cr–Zr Refractory High-Entropy Alloys fabricated via Powder Metallurgy
Near Net Shape Formation of High Entropy Carbide by Reactive Flash Sintering
Phase stability and local bonding in high entropy UHTC transition metal carbides
PhaseForge: Accelerating Phase Stability Predictions for Frontier Materials Without CALPHAD Databases
Powering Tomorrow with AI-Driven High-Entropy Discovery
Refractory Compositionally Complex Ceramics, Nanocrystalline Alloys, and Dual-Phase Composites: From Material Discovery to Innovative Processing
Refractory High-Entropy Alloys For Compact Fusion
Superior Spall Strength and Toughness in Hf₂₆Nb₂₀Ti₃₁V₂₃ Relative to Previously Tested Refractory Multi-Component Alloys
Swift Heavy Irradiation in Sr-Based High-Entropy Perovskites
Tailored Approaches to High-Temperature Deformation in Refractory Systems
Temperature Dependence of Yield Strength in NbTaTiV-Based Refractory Complex Concentrated Alloys
Tension-Compression Asymmetry in HfNbTaTiZr Refractory High-Entropy Alloys Studied with In Situ Neutron Diffraction
Thermal conductivity of high entropy ceramics before and after irradiation
Thermodynamics of Mechanical Behavior in R-CCAs: Balancing Room-Temperature Tensile Ductility and High Temperature Strength

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