| Abstract Scope |
Lithium batteries are among the promising next-generation energy storage devices due to their ultrahigh theoretical capacity and the lowest electrochemical potential. However, their applications remain hindered by unstable electrolyte–electrode interfaces, a narrow electrochemical window, and severe safety concerns.
A novel UV path to make electrolyte with enhanced electrochemical performance and safety. Films were synthesized via UV to form flexible Li⁺ interpenetrating networks. These networks enable the integration of ceramic structures within a polymer matrix, free-standing electrolyte films that combine mechanical flexibility with interfacial stability.
The resulting electrolyte exhibit valid electrochemical properties, high ion conductivity, wider (ESW), and lithium-ion transference number. The nanofillers plays an excellent role in stabilizing the SEI and suppress lithium dendrite formation. Cells demonstrated stable cycling without short-circuiT,the effectiveness of dendrite inhibition. full-cell showed cycling stability and high Coulombic efficiency.
UV-assisted electrolyte offers a promising pathway for the development of high-performance, safe, and scalable solid-state lithium batteries. |