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Meeting MS&T22: Materials Science & Technology
Symposium Emergent Materials under Extremes and Decisive In Situ Characterizations
Presentation Title In Situ Microstructural Characterization of Metallic Nuclear Fuels
Author(s) Tiankai Yao, Kaustubh Bawane, Sriram Vijayan, Amey Khanolkar, Fidelma Giulia Di Lemma , Lingfeng He
On-Site Speaker (Planned) Lingfeng He
Abstract Scope Metallic nuclear fuels are ideal for fast reactors because of higher densities of fissile and fertile materials than other fuel forms. The phase evolution and fuel-cladding chemical interaction in metallic fuels in nuclear reactor environments are not yet well understood. In this work, we design in situ transmission electron microscopy (TEM) experiments using a micro electromechanical system (MEMS) based heating stage and study microstructural evolution in two metallic fuel systems, U-Zr and U-Mo as a function of temperature. The thermally driven phase changes are characterized by using electron diffraction and ChemiSTEM techniques. We further modify MEMS-based heating stage to study thermal gradient effects on microstructural evolution in these metallic fuels. In addition, in situ laser ultrasonic measurements supplement in situ TEM characterization to monitor phase transitions during thermal processing. These in situ characterization experiments provide better mechanistic understanding in microstructural and chemical evolution in metallic fuels under non-equilibrium conditions.

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

Characterization of Disordered Oxides with Neutron Total Scattering
Determination of P-V Equation of State of a Natural Clinoptilolite Using High Pressure Synchrotron X-ray Diffraction
Electrochemical Deposition with Redox Replacement of Lanthanum with Uranium in Molten LiCl-KCl
In-Situ High Temperature Neutron and X-ray Studies of Corrosion Kinetics and Salt Properties
In Situ Microstructural Characterization of Metallic Nuclear Fuels
Influence of Cementite Morphology and Its Orientation on Deformation and Fracture of Pearlitic Steel Wire
Novel Automated Approaches for Studying Extended In Situ Mechanical and High Temperature Transformations of New Materials and Alloys in Scanning Electron and X-ray Microscopy
Opportunities in High-pressure Science Enabled by Next Generation Synchrotron Sources
Structural Transformations Induced under Coupled Extreme Conditions
The Role of Anisotropic Diffusion on the Bubble/Void Superlattice Formation in Metals
Understanding Surface Radiation Damage in Concentrated Solid-Solution Alloys by Nanoindentation
In-Situ X-ray Absorption Spectroscopy of Actinide Speciation in Aqueous Fluids at Extreme Conditions

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