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Meeting Materials Science & Technology 2012
Symposium International Symposium on Defects, Transport and Related Phenomena
Presentation Title Discerning the Size Effects on the Ionic Conductivity of Doped Ceria
Author(s) Robert Kasse, Kevin S. Jones, Juan C. Nino
On-Site Speaker (Planned) Juan C. Nino
Abstract Scope Lowering the operating temperature of solid oxide fuel cells (SOFCs) for use at intermediate temperatures (400-800°C), is important for the expansion of SOFC technology into automotive applications. Several strategies (multi-doping, microstructure control, etc.) have been proposed to increase the electrolyte conductivity and avoid unacceptable ohmic losses at these lower temperatures. However, depending on the literature that is followed, it is still unclear whether grain size reduction is beneficial for enhancing the ionic conductivity in rare earth doped ceria or not. This may be because separating the contributions from the grain and grain boundaries is difficult for polycrystalline samples (bulk and film). Also, data from thin films with varying thicknesses have mainly been collected from surface measurements, where surface and fringing field effects poses problems. Here we present maiden comprehensive work on Ce<sub>0.9</sub>Nd<sub>0.1</sub>O<sub>2-δ</sub> bulk and thin film electrolytes in an attempt to discern the size effects on conductivity.
Proceedings Inclusion? Undecided

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

A Simple Model for Determination of Grain Boundary Potential from Current-Voltage Characteristics
Atomic Resolution Imaging of Hf Segregation at Polycrystalline Alumina Grain Boundaries
Atomistic Simulations of Ceria Nanoparticles
Ceramic Defect Characterizations within Atomistic-Based Multiscale Analysis
Complete Representation of Ionic and Electronic Transport Properties of Mixed Ionic Electronic Conductors under Isothermal and Nonisothermal Conditions
Compositional Stability and Oxygen Exchange Kinetics of Oxide Hetero-Junction Electrodes
Correlations between Grain Boundary Fracture Behavior and Structure under Different Doping Conditions
Defect Structures in Ta- and Ti-Excess Zn2TiO4
Design of Spinel Oxides as Candidate p-Type Transparent Conductors
Discerning the Size Effects on the Ionic Conductivity of Doped Ceria
Effect of Dopants on Interdiffusion of Aluminum and Oxygen through Grain-boundaries in Polycrystalline Alumina
Exploring the Kinetics of Associated Defects in Ferroelectric Materials Using EPR and TSDC Techniques
First-Principles Density Functional Theory Study of Grain Boundary Diffusion in Alpha-Al2O3 Crystal
First-Principles Study of the Oxygen Evolution Reaction and Electronic Conductivity of Li2O2
Ionomigration of Second Phase Inclusions in 8YSZ under SOFC and SOEC conditions
Local and Defect Structure Analysis of ITO-alternative Crystalline and Non-crystalline Transparent Conducting Oxides (TCOs)
Microscopic Origin of the Large Electrostriction in Gd-Doped Ceria and Implications for Other Oxygen Ion Conductors
Microstructural Effects on Oxygen Surface Exchange of La0.6Sr0.4Co0.2Fe0.8O3 Thin Films
Non-Isothermal Mass/Charge Transport in Mixed Ionic Electronic Conductor, BaCo0.7Fe0.22Nb0.08O3-δ
Optical In-Situ Spectroscopy of Titania Thin Films
Oxygen Transport and Surface Exchange Kinetics of SOFC Cathode Materials
Parameterized Exploration of Multi-Species Transport Permeation in BZY20 Using Numerical Modeling
Point Defects and Transport in Transition Metal-Containing Orthosilicates
Secondary Transport Phenomena in Ceramic Membranes under Electrochemical Potential Gradients
SrTiO3 as Master Example of Nanosize Effects in Mixed Conducting Oxides
Surface Exchange in (La,Sr)MnO3 Films: Effects of Strain, Orientation, and Microstructure on Oxygen Reduction
Surface Protonics: Basicity and Proton Activity on Oxide Surface
TEM and CBED Techniques for the Study of Point Defect Structure of Single Crystal YAG Scintillators
Understanding Defect Behavior in Nuclear Energy Materials

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